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Highlights Establishes a unified framework linking the origins, descriptors, and catalytic functions of polarisation in covalent organic frameworks (COFs). Systematically categorises polarisation engineering strategies i...

Abstract Photo-redox catalysis has emerged as a new generation of biochemical protocols in proximity labeling, noninvasive therapy, ultrafast activation. However, the well-developed photocatalysts cannot simultaneously p...

Abstract FLPClusters, which are structurally precise metal clusters incorporating Frustrated Lewis Pairs (FLPs), represent a promising class of FLP catalysts. Although FLPClusters have emerged only recently, their precis...

In this study, we present an effective chemo-enzymatic method for synthesizing di- and tetra-carboxyl–functionalized poly(ethylene glycol)s (PEGs) using Candida antarctica lipase B (CALB). PEG-diacid was synthesized th...

Carbon capture, utilization, and storage (CCUS) technology is an essential component of China's strategy to achieve carbon neutrality. It represents the necessary pathway for near-zero emissions from fossil fuels and pro...

Abstract Herein, Ru⁰/TiO₂ nanocomposites containing 0.5 wt% Ru were prepared via a simple wet-impregnation route followed by chemical reduction and were thoroughly characterized by XRD, FTIR, SEM, TEM, and EDS analys...

Catalytic methane decomposition (CMD) offers a direct pathway to CO2-free hydrogen by converting CH4 into H2 and solid carbon. However, its application is constrained by the need for efficient heat delivery to the cataly...

Abstract Stomata of plant leaves open to enable CO2 entry for photosynthesis and close when CO2 in the leaf is elevated. CO2 is thought to promote stomatal closure in part by activating the SLAC1 anion channel at the gua...

Abstract Per- and polyfluoroalkyl substances (PFAS) and microplastics (MPs) are certain types of persistent plastic contaminants that are a cause of concern to both the ecosystems and human health. The nanotechnologies o...

The characteristic oral environment – with its dynamic clearance, moisture, microbial load, and inflammatory potential – makes oral diseases highly prevalent and therapeutically challenging. Metal-organic frameworks ...

ABSTRACT Pyroelectric catalysis has shown promising prospects for sustainable energy generation and medical treatments. However, its potential is limited by intrinsically low pyroelectric coefficients and insufficient in...

Abstract The dual challenges of waste biomass disposal and escalating contamination by inorganic, organic, and emerging microplastic pollutants demand sustainable, circular remediation strategies. Biochar, a carbon-rich,...

Interweaving boron with metal atoms within a two-dimensional plane represents a promising strategy to fabricate unconventional boron networks. However, the practical synthesis and structural determination of such materia...

The cytochrome P450 enzymes catalyze the hydroxylation of organic substrates by dioxygen. The high-potential reactive intermediate in cytochrome P450 catalysis, compound I (CI), has the capacity to deliver oxidizing equi...

The first NHC–Cu-catalyzed decomposition of formic acid (FA) is reported. In the presence of PhSiH3, only hydrogen is generated while CO2 is captured by a silane species. The decomposition of an equimolar mixture of FA...

As the global carbon crisis worsens, we need the technology which can evolve from capturing carbon to efficiently using it. Dielectric barrier discharge (DBD) systems under mild conditions, a type of non-thermal plasma (...

Abstract Direct hydrogenation of CO2 with renewable H2 into value-added chemicals provides a promising pathway for sustainable carbon utilization in the future. Although extensive research has been conducted on CO2 hydro...

Anions are ionic species that play important roles in biology, medicine, catalysis, and environmental science. Identifying these species is crucial for industrial applications and clinical diagnostics. In recent years, e...

Near-surface molecular-beam mass spectrometry (ns-MBMS) is a highly sensitive and non-destructive method for temporal monitoring of catalytic conversions on solid surfaces, yet not widely applied in heterogeneous catalys...

Porous ceramics are widely used in fields such as heat insulation, filtration, sound absorption, and catalysis due to their good chemical stability, as well as the high permeability and large specific surface area of por...

Abstract To interpret and transmit biological signals, proteins use correlated motions. Experimental determination of these dynamics and the structural distributions they generate remains a key challenge. Here, using 114...

The study explores an eco-efficient synthesis method for hydroxyapatite (HAP) from mineral residues rich in calcium carbonate (CaCO3) and monopotassium phosphate (KH2PO4). The process is based on a chemical reaction in a...

Abstract The catalytic decomposition of ammonia under mild conditions is a promising route for green hydrogen production. However, conventional dissociative ammonia decomposition pathways over metal sites are suffering f...