Quantitative measurement of spatial distribution of effective refractive index induced by local electron concentration at a nano slit

Surface plasmon polaritons (SPPs) have found their key applications in high-sensitivity biomolecular detection and integrated photonic devices for optical communication via light manipulation at nanostructures. Despite their broad utility, SPPs are known to be accompanied by other complex near-field propagation modes, such as quasi-cylindrical waves (QCWs) and composite diffracted evanescent waves (CDEWs), whose electromagnetic and quantum propagation effects have not been comprehensively understood especially regarding their mutual interaction with SPPs. In this study, we addressed this complexity by employing a nano groove structure and a high-stability broadband femtosecond laser as a light source, the spatial phase distribution around the nano slit edge was measured with relative stability of a 4.6 × 10−11 at an averaging time of 0.01 s. Through this spatial phase spectrum, we precisely measured the nonlinear distribution of effective refractive index changes with an amplitude of 10−2 refractive index units at the edge of the nano slit–groove structure. These results reveal that the near-field effects on local electron concentration induced by nanostructure’s discontinuity can be quantitatively measured, which can contribute to a deeper understanding of SPP phenomena in nanostructures for the optimal design and utilization of the SPP effects in diverse nano-plasmonic applications.