Janus aramid nanofiber aerogel incorporating plasmonic nanoparticles for high-efficiency interfacial solar steam generation

Interfacial solar steam generation (ISSG) is a novel and potential solution to global freshwater crisis. Here, based on a facile sol-gel fabrication process, we demonstrate a highly scalable Janus aramid nanofiber aerogel (JANA) as a high-efficiency ISSG device. JANA performs near-perfect broadband optical absorption, rapid photothermal conversion and effective water transportation. Owning to these features, efficient desalination of salty water and purification of municipal sewage are successfully demonstrated using JANA. In addition, benefiting from the mechanical property and chemical stability of constituent aramid nanofibers, JANA not only possesses outstanding flexibility and fire-resistance properties, but its solar steaming efficiency is also free from the influences of elastic deformations and fire treatments. We envision JANA provides a promising platform for mass-production of high-efficiency ISSG devices with supplementary capabilities of convenient transportation and long-term storage, which could further promote the realistic applications of ISSG technology.