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Dehydrogenation of Isopropanol on Copper-Containing Mesoporous Catalysts

Balsamo, Nancy Florentina et al · American Chemical Society · 2010

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Author / responsible party
Balsamo, Nancy Florentina et al
Publisher
American Chemical Society
Year
2010
ISSN
0888-5885
ISSN
0888-5885
Language
English

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Copper-containing mesoporous catalysts with an MCM-41 type structure have been prepared using direct hydrothermal synthesis and characterized using XRD, AAS, N2 adsorption-desorption, DRUV-vis, and TEM. All of the samples showed high structural regularity and surface area. Three copper species are presented in these materials: isolated mononuclear Cud+ species, oligonuclear [Cud+...Od-...Cud+]n clusters, and bulky CuO oxides. These materials were catalytically tested in isopropanol dehydrogenation, showing good activity and very high selectivity to propanone at 300 °C. A further reduction treatment of the samples allowed us to suggest possible active species. Both the [Cud+...Od-...Cud+]n clusters and the isolated Cud+ cations seem to be the species responsible for isopropanol dehydrogenation. Fil: Balsamo, Nancy Florentina. Universidad Tecnológica Nacional. Facultad Regional Córdoba; Argentina Fil: Chanquia, Corina Mercedes. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Tecnológica Nacional. Facultad Regional Córdoba; Argentina

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APA 7

Balsamo, N. F. E. A. (2010). Dehydrogenation of Isopropanol on Copper-Containing Mesoporous Catalysts. http://hdl.handle.net/11336/278372

MLA

Balsamo, Nancy Florentina et al. "Dehydrogenation of Isopropanol on Copper-Containing Mesoporous Catalysts." 2010. http://hdl.handle.net/11336/278372.

Chicago

Balsamo, Nancy Florentina et al. 2010. "Dehydrogenation of Isopropanol on Copper-Containing Mesoporous Catalysts.". http://hdl.handle.net/11336/278372.

Harvard

Balsamo, N. F. E. A. 2010, Dehydrogenation of Isopropanol on Copper-Containing Mesoporous Catalysts, American Chemical Society, available at: http://hdl.handle.net/11336/278372 [Accessed 7 Aug. 2026].

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Title
Dehydrogenation of Isopropanol on Copper-Containing Mesoporous Catalysts
Author / contributors
Balsamo, Nancy Florentina et al
Publisher
American Chemical Society
Publication year
2010
ISSN
0888-5885
ISSN
0888-5885
Language
English

Subjects

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DEHYDROGENATION; ISOPROPANOL; COPPER; NANOCATALYST; https://purl.org/becyt/ford/2.10; https://purl.org/becyt/ford/2
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